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Effects of the SAPO-11 synthetic process on dehydration of ethanol to ethylene

Lina WU, Xiaoxing SHI, Qun CUI, Haiyan WANG, He HUANG

《化学科学与工程前沿（英文）》 2011年第5卷第1期页码 60-66 doi: 10.1007/s11705-010-0540-7

摘要： The effects of the synthetic condition of SAPO-11 molecular sieves on ethanol dehydration to ethylene were studied. Product-compositions, ethanol conversion, and selectivity to ethylene of synthesized and commercial SAPO-11 molecular sieves were compared. Results are as follows: the optimal synthetic conditions for SAPO-11 molecular sieves are adding pseudoboehmite before orthophoshporic, using di-n- propylamine as the template, having a mass fraction of 40% colloidal silica as the silica source and the starting gel obtained, and running at 200°C for 48 h. From the patterns of NH -TPD, the amount of acid synthesized by SAPO-11 molecular sieves is less than that by commercial SAPO-11 molecular sieves, and has a stronger weak acid. Also, ethanol conversion and selectivity to ethylene reached 99% at 280°C on synthesized SAPO-11, lower by 20°C compared to commercial SAPO-11. For two SAPO-11 molecular sieves, the by-products in the gas phase are mainly ethane, propane, propene, isobutane, n-butane, propadiene, butylene and some higher hydrocarbons. The by-products in the liquid phase are ethyl ether and acetaldehyde.

关键词： SAPO-11 molecular sieves synthesis ethanol ethylene dehydration

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Removal efficiencies of natural and synthetic progesterones in hospital wastewater treated by different

《环境科学与工程前沿（英文）》 2022年第16卷第10期 doi: 10.1007/s11783-022-1558-z

摘要：

● The concentrations of 61 progesterones in HWW, PFTE, SBTE were evaluated.

关键词： Progesterones Hospital wastewater Primary filtration treatment effluent Secondary biological treatment effluent Disinfection process

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合成橡胶化学及技术进展

武冠英

《中国工程科学》 1999年第1卷第3期页码 79-85

摘要：

文章从合成橡胶的化学基础出发，叙述了合成橡胶工业二十世纪以来的过去、现状，并展望未来。着重讨论了合成化学基础及相应聚合工艺过程的进步这两方面的问题。指出合成橡胶化学基础中活性聚合、可控聚合，包括茂金属催化剂仍为近期的重点；气相聚合工艺将会得到较大的发展；高效聚合釜的研究仍是核心问题；环保问题应更受到重视。

关键词：合成橡胶合成化学活性/控制聚合气相聚合

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Performance of completely autotrophic nitrogen removal over nitrite process under different aeration

GUO Jinsong, YANG Guohong, FANG Fang, QIN Yu

《环境科学与工程前沿（英文）》 2008年第2卷第4期页码 439-445 doi: 10.1007/s11783-008-0046-4

摘要： In this study, three sequential batch biofilm reactors (SBBRs) were operated for 155 days to evaluate the performance of completely autotrophic nitrogen removal over nitrite (CANON) process under different aeration modes and dissolved oxygen (DO). Synthetic wastewater with 160-mg NH-N/L was fed into the reactors. In the continuously-aerated reactor, the efficiency of the ammonium nitrogen conversion and total nitrogen (TN) removal reached 80% and 70%, respectively, with DO between 0.8–1.0 mg/L. Whereas in the intermittently-aerated reactor, at the aeration/non-aeration ratio of 1.0, ammonium was always under the detection limit and 86% of TN was removed with DO between 2.0–2.5 mg/L during the aeration time. Results show that CANON could be achieved in both continuous and intermittent aeration pattern. However, to achieve the same nitrogen removal efficiency, the DO needed in the intermittently-aerated sequential batch biofilm reactor (SBBR) during the aeration period was higher than that in the continuously-aerated SBBR. In addition, the DO in the CANON system should be adjusted to the aeration mode, and low DO was not a prerequisite to CANON process.

关键词： Synthetic wastewater process Whereas biofilm detection

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Application of fuzzy analytic hierarchy process model on determination of optimized pile-type

Lei MA, Shuilong SHEN, Jinhui ZHANG, Yang HUANG, Feng SHI

《结构与土木工程前沿（英文）》 2010年第4卷第2期页码 252-257 doi: 10.1007/s11709-010-0017-2

摘要： Pile-type selection is a very important stage of foundation design, and there are many field factors influencing the decision of pile-type selection. Since there is a limitation of traditional “major factors method” to satisfy the requirement of modern foundation construction, this study presents an efficient approach, in which analytic hierarchy process (AHP) is employed. AHP is a multiple criteria decision-making tool that has been applied in many fields related to the decision-making, e.g., in the field of economics, marketing, sociology, etc. However, it is rarely reported that AHP is applied in the field of civil engineering for decision making. In this study, AHP combined with fuzzy synthetic evaluation method is employed to select the type of pile used as the foundation of a residential building in Fuzhou, Fujian Province, China. The results show that fuzzy AHP approach is an easy and efficient way for pile-type selection.

关键词： pile type fuzzy synthetic evaluation analytic hierarchy process (AHP) optimal selection

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Genome reprogramming for synthetic biology

Kylie Standage-Beier,Xiao Wang

《化学科学与工程前沿（英文）》 2017年第11卷第1期页码 37-45 doi: 10.1007/s11705-017-1618-2

摘要： The ability to go from a digitized DNA sequence to a predictable biological function is central to synthetic biology. Genome engineering tools facilitate rewriting and implementation of engineered DNA sequences. Recent development of new programmable tools to reengineer genomes has spurred myriad advances in synthetic biology. Tools such as clustered regularly interspace short palindromic repeats enable RNA-guided rational redesign of organisms and implementation of synthetic gene systems. New directed evolution methods generate organisms with radically restructured genomes. These restructured organisms have useful new phenotypes for biotechnology, such as bacteriophage resistance and increased genetic stability. Advanced DNA synthesis and assembly methods have also enabled the construction of fully synthetic organisms, such as J. Craig Venter Institute (JCVI)-syn 3.0. Here we summarize the recent advances in programmable genome engineering tools.

关键词： CRISPR genome engineering synthetic biology rational design

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Renewable synthetic fuel: turning carbon dioxide back into fuel

《能源前沿（英文）》 2022年第16卷第2期页码 145-149 doi: 10.1007/s11708-022-0828-6

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Carbon-coated lithium titanate: effect of carbon precursor addition processes on the electrochemical performance

Shilei Ding, Zelong Jiang, Jing Gu, Hongliang Zhang, Jiajia Cai, Dongdong Wang

《化学科学与工程前沿（英文）》 2021年第15卷第1期页码 148-155 doi: 10.1007/s11705-020-2022-x

摘要： In this paper, two carbon-coated lithium titanate (LTO-C1 and LTO-C2) composites were synthesized using the ball-milling-assisted calcination method with different carbon precursor addition processes. The physical and electrochemical properties of the as-synthesized negative electrode materials were characterized to investigate the effects of two carbon-coated LTO synthesis processes on the electrochemical performance of LTO. The results show that the LTO-C2 synthesized by using Li CO and TiO as the raw materials and sucrose as the carbon source in a one-pot method has less polarization during lithium insertion and extraction, minimal charge transfer impedance value and the best electrochemical performance among all samples. At the current density of 300 mA·h·g , the LTO-C2 composite delivers a charge capacity of 126.9 mA·h·g , and the reversible capacity after 300 cycles exceeds 121.3 mA·h·g in the voltage range of 1.0–3.0 V. Furthermore, the electrochemical impedance spectra show that LTO-C2 has higher electronic conductivity and lithium diffusion coefficient, which indicates the advantages in electrode kinetics over LTO and LTO-C1. The results clarify the best electrochemical properties of the carbon-coated LTO-C2 composite prepared by the one-pot method.

关键词： lithium titanate carbon-coated carbon precursor synthetic process

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Targeting “undruggable” c-Myc protein by synthetic lethality

Chen Wang, Hui Fang, Jiawei Zhang, Ying Gu

《医学前沿（英文）》 2021年第15卷第4期页码 541-550 doi: 10.1007/s11684-020-0780-y

摘要： Synthetic lethal screening, which exploits the combination of mutations that result in cell death, is a promising method for identifying novel drug targets. This method provides a new avenue for targeting “undruggable” proteins, such as c-Myc. Here, we revisit current methods used to target c-Myc and discuss the important functional nodes related to c-Myc in non-oncogene addicted network, whose inhibition may cause a catastrophe for tumor cell destiny but not for normal cells. We further discuss strategies to identify these functional nodes in the context of synthetic lethality. We review the progress and shortcomings of this research field and look forward to opportunities offered by synthetic lethal screening to treat tumors potently.

关键词： synthetic lethality undruggable transcription factor c-Myc

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Water-soluble BODIPY and aza-BODIPY dyes: synthetic progress and applications

Gang FAN,Le YANG,Zhijian CHEN

《化学科学与工程前沿（英文）》 2014年第8卷第4期页码 405-417 doi: 10.1007/s11705-014-1445-7

摘要： In recent years, boron-dipyrromethene (BODIPY) and boron-azadipyrromethene (aza-BODIPY) dyes have attracted considerable multidisciplinary attention due to their diverse applications. By introducing various hydrophilic groups, such as quaternary ammonium, sulfonate or oligo-ethyleneglycol moieties into the BODIPY core, the solubilities of these dyes in aqueous solution can be greatly improved while maintaining their high fluorescence quantum yields. Accordingly, applying these fluorescent dyes in aqueous systems to areas such as chemosensors, biomacromolecule labeling, bio-imaging and photodynamic therapy has been achieved. In this article, the recent progress on the synthesis, optical properties and application of water-soluble BODIPY dyes and aza-BODIPY dyes is reviewed.

关键词： boron-dipyrromethene boron-azadipyrromethene synthetic progress applications

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SCRaMbLE drive application of synthetic yeast genome

Jin Jin, Yuan Ma, Duo Liu

《化学科学与工程前沿（英文）》 2018年第12卷第4期页码 832-834 doi: 10.1007/s11705-018-1749-0

摘要：

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Hollow-fiber gas penetration electrodes efficiently produce renewable synthetic fuels

《能源前沿（英文）》 2022年第16卷第5期页码 700-705 doi: 10.1007/s11708-022-0842-8

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Cell-free systems in the new age of synthetic biology

Fernando Villarreal,Cheemeng Tan

《化学科学与工程前沿（英文）》 2017年第11卷第1期页码 58-65 doi: 10.1007/s11705-017-1610-x

摘要： The advent of synthetic biology has ushered in new applications of cell-free transcription-translation systems. These cell-free systems are reconstituted using cellular proteins, and are amenable to modular control of their composition. Here, we discuss the historical advancement of cell-free systems, as well as their new applications in the rapid design of synthetic genetic circuits and components, directed evolution of biomolecules, diagnosis of infectious diseases, and synthesis of vaccines. Finally, we present our vision on the future direction of cell-free synthetic biology.

关键词： cell-free system application

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polygeneration system of a combination of the gasified coal gas and the pyrolyzed coal gas to form the synthetic

Kechang XIE, Fan LI

《化学科学与工程前沿（英文）》 2010年第4卷第4期页码 383-384 doi: 10.1007/s11705-010-0526-5

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Flexural behavior of ECC hollow beams incorporating different synthetic fibers

Ahmmad A. ABBAS, Farid H. ARNA ’OT, Sallal R. ABID, Mustafa ÖZAKÇA

《结构与土木工程前沿（英文）》 2021年第15卷第2期页码 399-411 doi: 10.1007/s11709-021-0701-4

摘要： Twelve ECC beams with three different fiber types, along with four normal concrete beams, were tested in this study to evaluate the influence of cross-sectional hollowing on their flexural performance. The fiber types used were nylon monofilament (NM), low-cost untreated polyvinyl alcohol (PVA), and polypropylene (PP). Three different square hole sizes of 60, 80, and 100 mm with cross-sectional hollowing ratios of 0.16, 0.28, and 0.44, respectively, were adopted for each group of beams in addition to a solid beam. All beams were tested under four-point loading using a displacement-controlled testing machine. The test results showed that ECC beams can mostly withstand higher cracking and ultimate loads compared to their corresponding normal concrete versions. The results also showed that both the ductility and toughness of the ECC beams are higher than those of the normal concrete beams and that the ductility values of the hollow beams with a hole size of 60 mm are higher than those of the corresponding solid beams. Moreover, hollow ECC beams with hole sizes of 60 and 80 mm exhibited a higher ductility than a solid normal concrete beam.

关键词： hollow beam hollowing ratio ECC flexural strength ductility toughness